Project ’09- Fluorescent Nanowire Growth

William Neely

Mentored by: Bret Flanders

Frequency Combs ‘08

 

Welcome to my K-State Physics REU 2009 homepage. Here you can find out more about what I’m doing this summer along with information about myself and some useful links to help you understand what I’m doing. I will also try to keep a diary of what I have accomplished each day.

Project Goals: To grow a nanowire using the Directed Electrochemical Nanowire Assembly (DENA) technique that fluoresces when attaching to a biological cell.

Applications

Research Strategy: Started by reading an incredible number of papers. For those interested, the following papers are rather interesting:

                             Directional Growth of Polypyrrole and Polythiopene wires, Thapa, et al.

                             Directional Growth of metallic and polymeric nanowires, Thapa, et al.

                             Monitoring Protein-Polymer Conjugation by a Fluorogenic Cu(I)-Catalyzed Azide-Alkyne 1,3-Dipolar Cycloaddition, Dirks, et al.

                             A Stepwise Huisgen Cycloaddition Process: Copper(I)-Catalyzed Regioselective “Ligation” of Azides and Terminal Alkynes, Sharpless, et al.

                             Any paper on an electrochemically polymerized thin film.

                            

After buying the materials I tried to grow thin films of Poly(para-phenylene) (ppp) and 2-Aminofluorene (2AF). Both were successful but 2AF apparently doesn’t fluoresce L Currently trying to grow a wire of PPP.

                  

Also learned how to grow a nanowire using a solution of 10 mM EDOT (Ethylenedioxythiopene) and 20 mM SDS (Sodium Dodecyl Sulfate). Then learned how to grow films on glass slides using previous solution and a solution of 0.1M Pyrrole and 0.1M SDS. Lastly, learned how to create electrodes on slides by evaporating chromium and then gold onto the slide.

Research Progress:

                   Poly(para-phenylene):

                             Film grown, fluorescent spectra recorded

                             No nanowire growth

                   2-Aminofluorene (2AF)

                             Film grown, film is found to be non-fluorescent, the monoanion of 2AF is non-fluorescent even though the neutral and cation are fluorescent

                             No nanowire growth

                   PEG/Pyrrol Solution

                             Film grown, no readily available way to determine whether PEG was incorporated so project cut off

Final Presentation: Located here

Final Poster: On display in the hallowed hall of physics at Southwestern College. But an image of it is here.

Useful Terms:

            Nanowire

            Polymer

            Click-Chemistry

Useful Links: 

American Physical Society Statements on Ethics

American Institute of Physics

My Research group's home page

Funding:

This program is funded by the National Science Foundation through grant number PHY-0851599 <http://www.nsf.gov/awardsearch/showAward.do?AwardNumber=0851599.> .  Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation.

That is, to whoever reads this, thanks for the funding because the NSF is funded through your tax dollars. So it’s really you who we should be thanking.